Roadmap on exsolution for energy applications
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In: JPhys Energy, Vol. 5.2023, No. 3, 031501, 20.06.2023.
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TY - JOUR
T1 - Roadmap on exsolution for energy applications
AU - Neagu, Dragos
AU - Irvine, John T. S.
AU - Wang, Jiayue
AU - Yildiz, Bilge
AU - Opitz, Alexander Karl
AU - Fleig, Jürgen
AU - Wang, Yuhao
AU - Liu, Jiapeng
AU - Shen, Longyun
AU - Ciucci, Francesco
AU - Rosen, Brian A.
AU - Xiao, Yongchun
AU - Xie, Kui
AU - Yang, Guangming
AU - Shao, Zongping
AU - Zhang, Yubo
AU - Reinke, Jakob
AU - Schmauss, Travis A.
AU - Barnett, Scott A.
AU - Maring, Roelf
AU - Kyriakou, Vasileios
AU - Mushtaq, Usman
AU - Tsampas, Mihalis N.
AU - Kim, Youdong
AU - O’Hayre, Ryan
AU - Carrillo, Alfonso J.
AU - Ruh, Thomas
AU - Lindenthal, Lorenz
AU - Schrenk, Florian
AU - Rameshan, Christoph
AU - Papaioannou, Evangelos I.
AU - Kousi, Kalliopi
AU - Metcalfe, Ian S.
AU - Xu, Xiaoxiang
AU - Liu, Gang
N1 - Publisher Copyright: © 2023 Author(s). Published by IOP Publishing Ltd.
PY - 2023/6/20
Y1 - 2023/6/20
N2 - Over the last decade, exsolution has emerged as a powerful new method for decorating oxide supports with uniformly dispersed nanoparticles for energy and catalytic applications. Due to their exceptional anchorage, resilience to various degradation mechanisms, as well as numerous ways in which they can be produced, transformed and applied, exsolved nanoparticles have set new standards for nanoparticles in terms of activity, durability and functionality. In conjunction with multifunctional supports such as perovskite oxides, exsolution becomes a powerful platform for the design of advanced energy materials. In the following sections, we review the current status of the exsolution approach, seeking to facilitate transfer of ideas between different fields of application. We also explore future directions of research, particularly noting the multi-scale development required to take the concept forward, from fundamentals through operando studies to pilot scale demonstrations.
AB - Over the last decade, exsolution has emerged as a powerful new method for decorating oxide supports with uniformly dispersed nanoparticles for energy and catalytic applications. Due to their exceptional anchorage, resilience to various degradation mechanisms, as well as numerous ways in which they can be produced, transformed and applied, exsolved nanoparticles have set new standards for nanoparticles in terms of activity, durability and functionality. In conjunction with multifunctional supports such as perovskite oxides, exsolution becomes a powerful platform for the design of advanced energy materials. In the following sections, we review the current status of the exsolution approach, seeking to facilitate transfer of ideas between different fields of application. We also explore future directions of research, particularly noting the multi-scale development required to take the concept forward, from fundamentals through operando studies to pilot scale demonstrations.
KW - catalysis
KW - energy
KW - exsolution
KW - exsolved nanoparticles
KW - oxides
UR - http://www.scopus.com/inward/record.url?scp=85162693764&partnerID=8YFLogxK
U2 - 10.1088/2515-7655/acd146
DO - 10.1088/2515-7655/acd146
M3 - Article
AN - SCOPUS:85162693764
VL - 5.2023
JO - JPhys Energy
JF - JPhys Energy
SN - 2515-7655
IS - 3
M1 - 031501
ER -