TY - JOUR

T1 - Multidisciplinary Assessment of a Novel Carbon Capture and Utilization Concept including Underground Sun Conversion

AU - Zauner, Andreas

AU - Fazeni-Fraisl , Karin

AU - Wolf-Zöllner, Philipp

AU - Holzleitner, Marie-Theres

AU - Veseli , Argjenta

AU - Lehner, Markus

AU - Bauer, Stephan

AU - Pichler, Markus

N1 - Publisher Copyright: © 2022 by the authors. Licensee MDPI, Basel, Switzerland.

PY - 2022/1/29

Y1 - 2022/1/29

N2 - The current work investigates the feasibility of a novel Carbon Capture and Utilization (CCU) approach—also known as Underground Sun Conversion (USC) or geo-methanation. The overall objective of the current work is a comprehensive assessment on the technical, economic and legal aspects as well as greenhouse gas impacts to be concerned for establishing USC technology concept. This is achieved by applying multidisciplinary research approach combining process simulation, techno-economic and greenhouse gas assessment as well as legal analysis allows answering questions about technical, economic feasibility and greenhouse gas performance as well as on legal constraints related to large scale CCU using geo-methanation in depleted hydrocarbon reservoirs. CO2 from the industry and renewable H2 from the electrolyser are converted to geomethane in an underground gas storage and used in industry again to close the carbon cycle. Process simulation results showed the conversion rates vary due to operation mode and gas cleaning is necessary in any case to achieve natural gas grid compliant feed in quality. The geomethane production costs are found to be similar or even lower than the costs for synthetic methane from Above Ground Methanation (AGM). The GHG-assessment shows a significant saving compared to fossil natural gas and conventional power-to-gas applications. From a legal perspective the major challenge arises from a regulative gap of CCU in the ETS regime. Accordingly, a far-reaching exemption from the obligation to surrender certificates would be fraught with many legal and technical problems and uncertainties.

AB - The current work investigates the feasibility of a novel Carbon Capture and Utilization (CCU) approach—also known as Underground Sun Conversion (USC) or geo-methanation. The overall objective of the current work is a comprehensive assessment on the technical, economic and legal aspects as well as greenhouse gas impacts to be concerned for establishing USC technology concept. This is achieved by applying multidisciplinary research approach combining process simulation, techno-economic and greenhouse gas assessment as well as legal analysis allows answering questions about technical, economic feasibility and greenhouse gas performance as well as on legal constraints related to large scale CCU using geo-methanation in depleted hydrocarbon reservoirs. CO2 from the industry and renewable H2 from the electrolyser are converted to geomethane in an underground gas storage and used in industry again to close the carbon cycle. Process simulation results showed the conversion rates vary due to operation mode and gas cleaning is necessary in any case to achieve natural gas grid compliant feed in quality. The geomethane production costs are found to be similar or even lower than the costs for synthetic methane from Above Ground Methanation (AGM). The GHG-assessment shows a significant saving compared to fossil natural gas and conventional power-to-gas applications. From a legal perspective the major challenge arises from a regulative gap of CCU in the ETS regime. Accordingly, a far-reaching exemption from the obligation to surrender certificates would be fraught with many legal and technical problems and uncertainties.

UR - http://www.scopus.com/inward/record.url?scp=85123637441&partnerID=8YFLogxK

U2 - 10.3390/en15031021

DO - 10.3390/en15031021

M3 - Article

VL - 15.2022

JO - Energies : open-access journal of related scientific research, technology development and studies in policy and management

JF - Energies : open-access journal of related scientific research, technology development and studies in policy and management

SN - 1996-1073

IS - 3

M1 - 1021

ER -