Impact of annealing and hydrogenation on the superconducting transition temperature of (TiNbMoTaW)Nx high entropy alloy nitride films

Publikationen: Beitrag in FachzeitschriftArtikelForschung(peer-reviewed)

Autoren

  • Gabriel Pristáš
  • Július Bačkai
  • Filip Košuth
  • Radoven Bures
  • Mária Fáberová
  • Slavomír Gabáni
  • Oleksandr Onufriienko
  • Serhii Vorobiov
  • Karol Flachbart

Externe Organisationseinheiten

  • Slovak Academy of Sciences, Kosice
  • Slovak Academy of Sciences, Kosice

Abstract

Very recently it was shown that incorporation of nitrogen into Ti 0.2Nb 0.2Mo 0.2Ta 0.2W 0.2 high-entropy alloy films leads to a considerable superconducting transition temperature T C enhancement in corresponding (TiNbMoTaW) 1.0N x nitrides. Here we report, independently, about the impact of subsequent annealing and the influence of additional hydrogen incorporation on these films, which should lead to a further enhancement of T C. However, the expected T C increase was not observed, on the contrary, both annealing of films at 800 °C in vacuum and incorporation of hydrogen into these films led to a reduction of T C. Analysis of the results shows that in case of annealing this is related to nitrogen release from the films, in case of hydrogenation to reductions of the density of states at the Fermi level and of the electron-phonon interaction.

Details

OriginalspracheEnglisch
Aufsatznummer107851
Seiten (von - bis)1-7
Seitenumfang7
FachzeitschriftSolid State Sciences : SSS
Jahrgang161.2025
AusgabenummerMarch
DOIs
StatusVeröffentlicht - 1 Feb. 2025